W03 - Non-linear plasmon-exciton coupling in monolithic nanocrystals

Project description

In project W03, we aim to reveal the mechanisms of nonlinear exciton-plasmon coupling in the monolithic system copper monosulfide (CuS), which combines in one nano unit excitonic and plasmonic transitions in spectral vicinity. Our goal is to enhance nonlinear optical phenomena to a maximum by systematically modifying shape, size, and geometry of sheet-like CuS nanocrystals. Steady-state and time-resolved spectroscopy will be employed to study the photoluminescence for nonlinear excitation. A systematic experimental study will be flanked by theoretical efforts, unravelling the fundamental mechanisms and efficient strategies for near-infrared light harvesting based on surface plasmon-induced phenomena.

Cooperation projects

S01, S03, S04, S05, S06, W01, W02, W04, W05, W06, W07

Publications

  • Tailoring Charge Donor-Acceptor Interaction in CsPbBr3 Perovskite Nanocrystals through Ligand Exchange
    S.A.B. Shah, S. Ghimire, R. Lesyuk, M.V. Diamanti, V. Lughi and C. Klinke
    Small Science, 202300348 (2024, early view)
     
  • Shape- and excitation-dependent charge-carrier dynamics in colloidal MAPbI perovskites as nanostripes, nanosheets and nanoplatelets
    E. Klein, C. Rehhagen, R. Lesyuk, and C. Klinke
    J. Mater. Chem. C 11(28), 9495-9503 (2023)
     
  • Order-Invariant Two-Photon Quantum Correlations in PT-Symmetric Interferometers
    T. A. W. Wolterink, M. Heinrich, S. Scheel and A. Szameit
    ACS Photonics, 10(10), 3451-3457 (2023)
     
  • Synthesis, optoelectronic properties, and charge carrier dynamics of colloidal quasi-two-dimensional Cs3Bi2I9 perovskite nanosheets
    S. Ghimire, C. Rehhagen, S. Fiedler, U. Parekh, R. Lesyuk, S. Lochbrunner and C. Klinke
    Nanoscale 15(5), 2096-2105 (2023)
     
  • Template-Mediated Formation of Colloidal Two-Dimensional Tin Telluride Nanosheets and the Role of the Ligands
    F.G. He, E. Klein, S. Bartling, S. Saeidpour, B. Corzilius, R. Lesyuk and C. Klinke
    J. Phys. Chem. C 126(48), 20498–20504 (2022)
     
  • A braid for light
    S. Scheel and A. Szameit 
    Nature Photonics 16(5), 344-345 (2022)
     
  • Role of Magnetic Coupling in Photoluminescence Kinetics of Mn2+-Doped ZnS Nanoplatelets
    L. Dai, A. Torche, C. Strelow, T. Kipp, T. H. Vuong, J. Rabeah, K. Oldenburg, G. Bester, A. Mews, C. Klinke and R. Lesyuk
    ACS Appl. Mater. Interfaces 14(16), 18806-18815 (2022)
     
  • Structural Reconstruction in Lead-Free Two-Dimensional Tin Iodide Perovskites Leading to High Quantum Yield Emission
    S. Ghimire, K. Oldenburg, S. Bartling, R. Lesyuk and C. Klinke
    ACS Energy Lett. 7(3), 975-983 (2022)

Project leaders

Dr. Rostyslav Lesyuk
Phone: +49 (0)381 498 6865
Email: rostyslav.lesyukuni-rostockde

Prof. Stefan Scheel
Phone: +49 (0)381 498 6920
Email: stefan.scheeluni-rostockde

Institution

University of Rostock
Institute of Physics
Albert-Einstein-Str. 23
18059 Rostock